I fear the setup may prove dubious (it looks like 6 or 7 dependencies alone are needed, and if any version of any item was not compatible with the rest, I could be spinning my wheels) so I suppose I will wait and hope the situation with Debian and GTK 4 changes.
The package name is misleading, libgtk-4 is the real name of the package and the -1 is the version of the package in Debian. libgtk-4-1 will actually install the 4.0 series, and libgtk-4-0 is the 3.99 series.